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Charge transfer and slow magnetic relaxation in a series of cyano-bridged FeIII4MII2 (M = Fe II , Co II , Ni II ) molecules

https://doi.org/10.1039/c8qi01245h

Wang, Jin-Hua ; Vignesh, Kuduva R. ; Zhao, Jia ; Li, Zhao-Yang ; Dunbar, Kim R. ( February 2019 , Inorganic Chemistry Frontiers)

The synthesis, single-crystal structures and magnetic properties of three new cyano-bridged complexes [FeIII4MII2] (M = Fe II , Co II , Ni II ) are reported. Electronic absorption spectroscopy reveals the occurrence of intervalence charge transfer for [FeIII4FeII2]. Field-induced slow magnetic relaxation behavior is exhibited for [FeIII4CoII2] and [FeIII4NiII2] which originates from the ferromagnetic interactions between Fe III and M II spin centers of the square.
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